Materials

Active materials for experiments 001–007, with firing reference, clay composition guide, shopping list, and future process materials.

Clay body

MaterialSupplierUseNotes
Witgert 5041-25 Gietkleipoeder 300De Hazelaar / WitgertBase material — all current experimentsRed earthenware. SiO₂ 68.7%, Al₂O₃ 18.3%, Fe₂O₃ 5.2%, LOI 5.0%. Fire 950–1100°C oxidation. ~5–7% total shrinkage.

Binder

MaterialSupplierUseNotes
Agar agar powder (food-grade)Albert Heijn / onlineAgar gelcasting (exp-004, 005)1–3 wt% of agar/water solution. Dissolve >85°C, gels <35°C. Thermoreversible. Burns out 250–350°C cleanly.
Corn starchAlbert HeijnStarch consolidation (exp-002, 003)7–10 wt% of dry ceramic. Gelatinises >80°C. Burns out 300–500°C. Zero cost.

Slip additive

MaterialSupplierUseNotes
Darvan 811Seladon.be / ceramic suppliersDeflocculant for all slip casting0.3–0.6 ml per 100g dry ceramic. Keeps slip fluid at high solids loading (55–65 wt%). Do not exceed — causes flocculation above optimum.
Silica flour, 200 meshDe HazelaarBody filler in all slip formulas10 wt% of dry ceramic. Improves fired density and reduces shrinkage variation.
PVA (polyvinyl alcohol)Lab / craft supplier / Amazon.nlGreen body binder — freeze casting (exp-006, 007)0.5–1 wt% of dry ceramic. Dissolved in water before slip prep. Bridges particles after ice sublimation — without it, freeze-cast green bodies are extremely fragile. Burns out 250–350°C cleanly. Not needed for agar or starch experiments.
Methylcellulose (MC)Food supplier (e.g. Sosa, Texturas) / lab supplierAlternative green body binder — freeze casting; also relevant for extrusion0.5–2 wt% of dry ceramic. Less toxic than PVA, biodegradable, cellulose-derived. Reverse-gelling: dissolves in cold water, gels >60°C. Interchangeable with PVA at similar concentrations. Burns out 250–400°C. Available cheaply from molecular gastronomy suppliers.
GlycerolPharmacy / lab supplier / Amazon.nlIce crystal modifier — freeze castingGets excluded from the ice front as crystals grow, altering local growth kinetics and lamellar spacing. Non-toxic, food-safe. Try 0.5–2 wt% of slip. Also a mild plasticiser for the binder phase.
PEG (polyethylene glycol, MW 400–1000)Lab supplier / Amazon.nlBinder + ice crystal modifier — freeze castingWidely used in freeze casting literature as a dual-function additive. Low MW PEG (400) is liquid at RT; higher MW is waxy solid. 0.5–2 wt%. Modifies crystal morphology and bridges particles in green body.
Sucrose (table sugar)Albert Heijn — effectively freeMild ice crystal modifier — freeze castingSmall molecules get partially excluded from ice front, mildly altering crystal morphology at 1–5 wt%. Effect is subtle but non-zero and cost is zero. Worth including in a test run for comparison.
TPM (tripropylene glycol monomethyl ether, Dowanol TPM)Chemical / coating supplier (e.g. Sigma-Aldrich, VWR)Cosolvent + ice crystal modifier — freeze castingUsed in combination with PVA + water in freeze casting slip. Acts as cosolvent: depresses freezing point slightly and gets excluded from the advancing ice front, enriching the liquid interlayer between crystals. Results in finer, more controlled lamellar pore structures. Relatively low toxicity for a glycol ether. Typical use 2–10 wt% of water phase. Removed during sublimation/freeze drying along with water.
CuCl₂·2H₂O (copper chloride dihydrate)Lab / chemistry supplierAPD additive — freeze casting (exp-006, 007)Optional. 1 wt% of slip. Per Wu et al. (2023) — promotes liquid-phase structure preservation during ambient-pressure drying. Effect on clay (vs. fine alumina) is speculative.

Mold material

MaterialSupplierUseNotes
Platinum-cure silicone, Shore A30 (Mold Max 30)FormX.nlFlexible two-part molds — all gelcasting experimentsShore A30 is soft enough for undercuts, rigid enough to hold fine detail. 500g kit makes one ribbed tile mold. Life: 20–100 pours. Best option for fine features and fragile green bodies.
PCL pellets (polycaprolactone) — bulkAliExpress / Amazon.nlThermoplastic rigid molds (simple geometries)Softens at 60°C in hot water, moldable by hand, sets rigid at room temp. Reusable indefinitely. ~€15–20/kg bulk. Same base material as Green Stuff World Flexi Mold. NOT flexible — design split molds with no undercuts. Avoid for fragile green bodies.
"Oogoo" DIY silicone (silicone caulk + cornstarch)Gamma / Praxis (neutral-cure caulk)Cheap flexible molds for simple shapesMix 100% neutral-cure silicone caulk + cornstarch 3:1 by weight. Press around master, sets flexible in ~30 min. ~€5–8 per mold. Flexible like silicone — peel-able. Lower detail and shorter life than Mold Max 30. Good for quick prototyping.
Copper sheet, 3mmMetal supplier / Amazon.nlCold-side thermal conductor — freeze casting (exp-006, 007)High conductivity needed for directional freezing. 150×150mm for exp-006, 100×100mm for exp-007.
PVC pipe (Ø50mm and Ø30mm)Gamma / PraxisCylindrical molds for freeze-cast specimensCut to 40mm (Ø50) and 20mm (Ø30) sections. Sealed to copper with silicone sealant.

Finish

MaterialSupplierUseNotes
Engobe (slip coating)Ceramic supplierSurface colour / texture before firingApplied to leather-hard or dry greenware. Cone 06–04.
Transparent glazeCeramic supplierWeatherproofing and aestheticsCone 06–04 (990–1060°C) for terracotta. Not required for feasibility experiments.

Firing Reference

Standard terracotta curve — total cycle 14–24h

PhaseRateRangeNotes
Initial heat-up30°C/hRT → 120°CFree water removal
Dehydration60°C/h120°C → 350°CBound water + binder burnout
Burnout soakHold 30 min350°CComplete organic burnout
Quartz zone ⚠50°C/h350°C → 650°CCritical: quartz inversion at 573°C (~2% volume change)
Main heat-up100–150°C/h650°C → 1080°C
Peak soakHold 1–2h1000–1080°CUniform sintering
Initial cool80°C/hPeak → 650°C
Quartz cool ⚠50°C/h650°C → 500°CJust as critical in reverse
Final cool100–200°C/h500°C → RT

Clay Composition Guide

How oxide analysis affects slip and fired properties — reference for Witgert 5041-25 and future clay choices

OxideWitgert valueEffect on fired bodyEffect on slip
SiO₂ (68.7%)HighLower vitrification temp, more glassy body; quartz inversion at 573°C governs firing curveLittle direct effect
Al₂O₃ (18.3%)ModerateMore refractory and stronger; too much → underfired at 1000°CLess plastic; needs more deflocculant
Fe₂O₃ (5.2%)Typical earthenwareRed/brown colour in oxidation; lowers vitrification slightlyLittle effect on viscosity
Fluxes — K₂O 2.3%, Na₂O 0.2%, CaO 0.2%, MgO 0.4%Low-moderatePromote densification and glass phase; CaO can cause lime popping if coarseAlkalis increase deflocculation sensitivity
LOI (5.0%)NormalOrganics burn out 300–600°C; fast firing traps gas → bloating or black coreN/A — measured on dry powder

Shopping List

Everything needed to run experiments 001–007 and all testing procedures. Items you likely already own (oven, freezer, pot, camera) are excluded.

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Future Process Materials

Materials for processes not yet in active experiments — LPCIM, geopolymer, and advanced mold systems.